Electrocatalytic CO2 reduction with an immobilized iron complex on gas diffusion electrodes

Open Access
Authors
Publication date 18-09-2025
Journal Chemical Communications
Volume | Issue number 61 | 76
Pages (from-to) 14693-14696
Number of pages 4
Organisations
  • Faculty of Science (FNWI) - Van 't Hoff Institute for Molecular Sciences (HIMS)
Abstract

The immobilization of molecular electrocatalysts on gas diffusion electrodes (GDEs) overcomes mass transport limitations inherent to solution-phase CO2 reduction. We report the immobilization of the molecular FeTDHPP catalyst on a GDE via supramolecular π-π interactions, achieving a 50-fold catalytic activity increase compared to solution-phase performance.

Document type Article
Note With supplementary file.
Language English
Published at https://doi.org/10.1039/d5cc01220a
Other links https://www.scopus.com/pages/publications/105016482020
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d5cc01220a (Final published version)
Supplementary materials
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