Two-step photoinduced charge separation and unexpectedly fast one-step charge recombination in a linked Donor2-Donor1-Acceptor system

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Authors
Publication date 1993
Journal Chemical Physics Letters
Volume | Issue number 214 | 5
Pages (from-to) 502-506
Organisations
  • Faculty of Science (FNWI) - Van 't Hoff Institute for Molecular Sciences (HIMS)
Abstract Photoinduced sequential two-step electron transfer occurs upon excitation of the 1,3-diphenylpropanedioato boron oxalate electron acceptor in a novel trichromophoric donor2-donor1-acceptor (D2-D1-A) system. The D2-D+1-A- state is fluorescent, while the D+2-D1-A- state is observed by transient absorption. The final giant dipole state, which is formed in ? 90% yield, is remarkably short-lived.
Document type Article
Published at https://doi.org/10.1016/0009-2614(93)85673-C
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