Finite-size effects in the nonphononic density of states in computer glasses

Open Access
Authors
Publication date 03-2020
Journal Physical Review E
Article number 032120
Volume | Issue number 101 | 3
Number of pages 5
Organisations
  • Faculty of Science (FNWI) - Institute of Physics (IoP) - Institute for Theoretical Physics Amsterdam (ITFA)
Abstract

The universal form of the density of nonphononic, quasilocalized vibrational modes of frequency ω in structural glasses, D(ω), was predicted theoretically decades ago, but only recently revealed in numerical simulations. In particular, it has been recently established that, in generic computer glasses, D(ω) increases from zero frequency as ω4, independent of spatial dimension and of microscopic details. However, it has been shown [Lerner and Bouchbinder, Phys. Rev. E 96, 020104(R) (2017)2470-004510.1103/PhysRevE.96.020104] that the preparation protocol employed to create glassy samples may affect the form of their resulting D(ω): glassy samples rapidly quenched from high-temperature liquid states were shown to feature D(ω)∼ωβ with β < 4, presumably limiting the degree of universality of the ω4 law. Here we show that exponents β < 4 are seen only in small glassy samples quenched from high-temperature liquid states - whose sizes are comparable to or smaller than the size of the disordered core of soft quasilocalized vibrations - while larger glassy samples made with the same protocol feature the universal ω4 law. Our results demonstrate that observations of β < 4 in the nonphononic density of states stem from finite-size effects, and we thus conclude that the ω4 law should be featured by any sufficiently large glass quenched from a melt.

Document type Article
Note ©2020 American Physical Society
Language English
Published at https://doi.org/10.1103/PhysRevE.101.032120
Other links https://www.scopus.com/pages/publications/85082666738
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PhysRevE.101.032120 (Final published version)
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