N-heterocyclic carbene IrCp*LX₂ molecular water oxidation catalysis; mechanistic insights and immobilization strategies

Authors	J.M. Koelewijn
Supervisors	J.N.H. Reek
Cosupervisors	R.J. Detz
Award date	29-03-2016
ISBN	9789402800678
Number of pages	200
Organisations	Faculty of Science (FNWI) - Van 't Hoff Institute for Molecular Sciences (HIMS)
Document type	PhD thesis
Note	Research conducted at: Universiteit van Amsterdam
Language	English
Downloads	Summary for UvA-DARE Thesis (complete) Front matter Chapter 1: The artificial leaf; a potential route towards sustainable energy applications Chapter 2: Reaction progress kinetic analysis as tool to reveal ligand effects in Ce(IV)-driven IrCpLX₂ catalyzed water oxidation Chapter 3: Photooxidation of a NHC IrCpCl₂ water oxidation catalyst by a Pt(II)-porphyrin sensitizer co-immobilized on FTO/TiO₂ photoanodes. Towards photodriven electrocatalytic oxidation of H₂O Chapter 4: Anode preparation strategies for the electrocatalytic oxidation of water based on strong MWCNT/Pyr⁺ interactions in aqueous solutions Chapter 5: Application of FTO/MWCNT/MxOy composite anodes prepared via electrophoretic deposition using sodium 1-pyrene sulphonate. Towards optimization of charge carrier transport in WOC/dye sensitized photoanodes Chapter 6: Oxidized porous silicon as a mesoporous support for an iridium based molecular water oxidation catalyst Summary / Samenvatting Back matter
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